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dc.contributor.authorGañán-Calvo, Alfonso M.-
dc.contributor.authorChapman, Henry N.-
dc.contributor.authorHeymann, Michael-
dc.contributor.authorWiedorn, Max O.-
dc.contributor.authorKnoska, Juraj-
dc.contributor.authorGañán-Riesco, Braulio-
dc.contributor.authorLópez-Herrera, José M.-
dc.contributor.authorCruz-Mazo, Francisco-
dc.contributor.authorHerrada, Miguel A.-
dc.contributor.authorMontanero, José M.-
dc.contributor.authorBajt, Saša-
dc.date.accessioned2023-08-10T12:43:44Z-
dc.date.available2023-08-10T12:43:44Z-
dc.date.issued2021-
dc.identifier.issn2073-4352-
dc.identifier.other1857864131-
dc.identifier.urihttp://nbn-resolving.de/urn:nbn:de:bsz:93-opus-ds-134315de
dc.identifier.urihttp://elib.uni-stuttgart.de/handle/11682/13431-
dc.identifier.urihttp://dx.doi.org/10.18419/opus-13412-
dc.description.abstractOne of the most successful ways to introduce samples in Serial Femtosecond Crystallography has been the use of microscopic capillary liquid jets produced by gas flow focusing, whose length-to-diameter ratio and velocity are essential to fulfill the requirements of the high pulse rates of current XFELs. In this work, we demonstrate the validity of a classical scaling law with two universal constants to calculate that length as a function of the liquid properties and operating conditions. These constants are determined by fitting the scaling law to a large set of experimental and numerical measurements, including previously published data. Both the experimental and numerical jet lengths conform remarkably well to the proposed scaling law. We show that, while a capillary jet is a globally unstable system to linear perturbations above a critical length, its actual and shorter long-term average intact length is determined by the nonlinear perturbations coming from the jet breakup itself. Therefore, this length is determined solely by the properties of the liquid, the average velocity of the liquid and the flow rate expelled. This confirms the very early observations from Smith and Moss 1917, Proc R Soc Lond A Math Phys Eng, 93, 373, to McCarthy and Molloy 1974, Chem Eng J, 7, 1, among others, while it contrasts with the classical conception of temporal stability that attributes the natural breakup length to the jet birth conditions in the ejector or small interactions with the environment.en
dc.description.sponsorshipMinisterio de Economía y Competitividadde
dc.description.sponsorshipDeutsche Forschungsgemeinschaftde
dc.language.isoende
dc.relation.uridoi:10.3390/cryst11080990de
dc.rightsinfo:eu-repo/semantics/openAccessde
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/de
dc.subject.ddc530de
dc.subject.ddc570de
dc.titleThe natural breakup length of a steady capillary jet : application to serial femtosecond crystallographyen
dc.typearticlede
dc.date.updated2021-09-13T16:46:13Z-
ubs.fakultaetEnergie-, Verfahrens- und Biotechnikde
ubs.fakultaetFakultätsübergreifend / Sonstige Einrichtungde
ubs.institutInstitut für Biomaterialien und biomolekulare Systemede
ubs.institutFakultätsübergreifend / Sonstige Einrichtungde
ubs.publikation.seiten13de
ubs.publikation.sourceCrystals 11 (2021), No. 990de
ubs.publikation.typZeitschriftenartikelde
Enthalten in den Sammlungen:04 Fakultät Energie-, Verfahrens- und Biotechnik

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