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Author: search.filters.author.Meinert, Florian

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    Dynamics of atoms within atoms
    (2022) Tiwari, Shiva; Engel, Felix; Wagner, Marcel; Schmidt, Richard; Meinert, Florian; Wüster, Sebastian
    Recent experiments with Bose–Einstein condensates have entered a regime in which thousands of ground-state condensate atoms fill the Rydberg-electron orbit. After the excitation of a single atom into a highly excited Rydberg state, scattering off the Rydberg electron sets ground-state atoms into motion, such that one can study the quantum-many-body dynamics of atoms moving within the Rydberg atom. Here we study this many-body dynamics using Gross-Pitaevskii and truncated Wigner theory. Our simulations focus in particular on the scenario of multiple sequential Rydberg excitations on the same rubidium condensate which has become the standard tool to observe quantum impurity dynamics in Rydberg experiments. We investigate to what extent such experiments can be sensitive to details in the electron–atom interaction potential, such as the rapid radial modulation of the Rydberg molecular potential, or p-wave shape resonance. We demonstrate that both effects are crucial for the initial condensate response within the Rydberg orbit, but become less relevant for the density waves emerging outside the Rydberg excitation region at later times. Finally we explore the local dynamics of condensate heating. We find that it provides only minor corrections to the mean-field dynamics. Combining all these insights, our results suggest Bose–Einstein condensates as a viable platform for the in situ and real time interrogation of ultra-cold chemistry dynamics involving Rydberg states.
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    Long-lived circular Rydberg qubits of alkaline-earth atoms in optical tweezers
    (2024) Hölzl, Christian; Götzelmann, Aaron; Pultinevicius, Einius; Wirth, Moritz; Meinert, Florian
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    In situ observation of chemistry in Rydberg molecules within a Bose-Einstein-condensate
    (2024) Engel, Felix; Tiwari, Shiva; Pfau, Tilman; Wüster, Sebastian; Meinert, Florian
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    Vibrational quenching of weakly bound cold molecular ions immersed in their parent gas
    (2020) Jachymski, Krzysztof; Meinert, Florian
    Hybrid ion–atom systems provide an excellent platform for studies of state-resolved quantum chemistry at low temperatures, where quantum effects may be prevalent. Here we study theoretically the process of vibrational relaxation of an initially weakly bound molecular ion due to collisions with the background gas atoms. We show that this inelastic process is governed by the universal long-range part of the interaction potential, which allows for using simplified model potentials applicable to multiple atomic species. The product distribution after the collision can be estimated by making use of the distorted wave Born approximation. We find that the inelastic collisions lead predominantly to small changes in the binding energy of the molecular ion.