Universität Stuttgart

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    Electro-active metaobjective from metalenses-on-demand
    (2022) Karst, Julian; Lee, Yohan; Floess, Moritz; Ubl, Monika; Ludwigs, Sabine; Hentschel, Mario; Giessen, Harald
    Switchable metasurfaces can actively control the functionality of integrated metadevices with high efficiency and on ultra-small length scales. Such metadevices include active lenses, dynamic diffractive optical elements, or switchable holograms. Especially, for applications in emerging technologies such as AR (augmented reality) and VR (virtual reality) devices, sophisticated metaoptics with unique functionalities are crucially important. In particular, metaoptics which can be switched electrically on or off will allow to change the routing, focusing, or functionality in general of miniaturized optical components on demand. Here, we demonstrate metalenses-on-demand made from metallic polymer plasmonic nanoantennas which are electrically switchable at CMOS (complementary metal-oxide-semiconductor) compatible voltages of ±1 V. The nanoantennas exhibit plasmonic resonances which can be reversibly switched ON and OFF via the applied voltage, utilizing the optical metal-to-insulator transition of the metallic polymer. Ultimately, we realize an electro-active non-volatile multi-functional metaobjective composed of two metalenses, whose unique optical states can be set on demand. Overall, our work opens up the possibility for a new level of electro-optical elements for ultra-compact photonic integration.
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    ItemOpen Access
    Femtosecond direct laser writing of conductive and electrically witchable PEDOT:PSS optical nanostructures
    (2025) Ludescher, Dominik; Ruchka, Pavel; Siegle, Leander; Huang, Yanzhe; Flad, Philipp; Ubl, Monika; Ludwigs, Sabine; Hentschel, Mario; Giessen, Harald
    Microscale three‐dimensional (3D)‐printing, with its remarkable precision and ability to create complex structures, has transformed a wide range of applications, from micro‐optics and photonics to endoscopy and quantum technologies. In these fields, miniaturization plays a crucial role in unlocking new capabilities. However, despite these advancements, most 3D‐printed optical structures have remained static, lacking dynamic behavior and tunability. In this study, a novel approach is presented that combines direct laser writing with the electrically switchable optical properties of the conductive polymer poly(3,4‐ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS). This integration facilitates the creation of dynamic structures directly on 3D‐printed objects, marking a significant step toward adaptive optical devices. The fabrication of electrically tunable structures is demonstrated via direct laser writing using PEDOT:PSS on indium tin oxide (ITO)‐coated glass substrates, as well as beneath and atop static 3D‐printed structures. It is found that electrical conductivity as well as the greyscale behavior of PEDOT:PSS remains intact after direct laser writing. The switching speed, durability, and gradual tunability of the material are explored upon complementary metal‐oxide‐semiconductor (CMOS)‐compatible voltages ranging from -3 to +2 V. In the future, this advancement opens exciting possibilities in adaptive micro‐optics, such as switchable apertures printed directly onto micro‐optical lenses.
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    ItemOpen Access
    Electrically switchable metallic polymer metasurface device with gel polymer electrolyte
    (2023) Jong, Derek de; Karst, Julian; Ludescher, Dominik; Floess, Moritz; Moell, Sophia; Dirnberger, Klaus; Hentschel, Mario; Ludwigs, Sabine; Braun, Paul V.; Giessen, Harald
    We present an electrically switchable, compact metasurface device based on the metallic polymer PEDOT:PSS in combination with a gel polymer electrolyte. Applying square-wave voltages, we can reversibly switch the PEDOT:PSS from dielectric to metallic. Using this concept, we demonstrate a compact, standalone, and CMOS compatible metadevice. It allows for electrically controlled ON and OFF switching of plasmonic resonances in the 2-3 µm wavelength range, as well as electrically controlled beam switching at angles up to 10°. Furthermore, switching frequencies of up to 10 Hz, with oxidation times as fast as 42 ms and reduction times of 57 ms, are demonstrated. Our work provides the basis towards solid state switchable metasurfaces, ultimately leading to submicrometer-pixel spatial light modulators and hence switchable holographic devices.