Browsing by Author "Rietdorf, Chantal"

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Open Access
Cradle-to-gate life cycle assessment of cylindrical sulfide-based solid-state batteries
(2024) Rietdorf, Chantal; De la Rúa, Cristina; Kiemel, Steffen; Miehe, Robert
PurposeSolid-state batteries (SSBs) are a current research hotspot, as they are safer and have a higher energy density than state-of-the-art lithium-ion batteries (LIBs). To date, their production only occurs on a laboratory scale, which provides a good opportunity to analyze the associated environmental impacts prior to industrialization. This paper investigates the environmental impacts of the production of cylindrical SSB, to identify environmental hotspots and optimization potentials.MethodsHere, an attributional cradle-to-gate life cycle assessment (LCA) is performed, focusing on SSBs that use a NMC811/lithium germanium phosphorous sulfide (LiGPS) composite cathode, a sulfide-based solid separator electrolyte, and a lithium metal anode. The life cycle impact assessment (LCIA) is performed in Umberto 11 using the Environmental Footprint 3.1 method with primary and literature data and the Evoinvent 3.9 database for background data.Results and discussionThe results show climate change impacts of 205.43 kg CO2 eq./kwh (for the base case), with hotspots primarily attributable to the electrolyte and cathode production, and more specifically to the LiPS and LiGPS synthesis as well as to the cathode active material. Additionally, the scenario analysis shows that an upscaling of the LiPS and LiGPS synthesis reduces environmental impacts across all assessed impact categories. In addition, it was shown that the use of an in situ anode further improves the overall environmental performance, while the use of alternative cathode active materials, such as NMC622 and LFP did not lead to any improvements, at least with reference to the storage capacity.ConclusionThe article highlights the environmental hotspots of sulfide-based SSB production, namely electrolyte and catholyte synthesis. The results show that upscaling the synthesis reduces the environmental impact and that cells with higher energy density show a favorable environmental performance. However, SSBs are still in the development stage and no final recommendation can be made at this time.
Open Access
How to simplify life cycle assessment for industrial applications : a comprehensive review
(2022) Kiemel, Steffen; Rietdorf, Chantal; Schutzbach, Maximilian; Miehe, Robert
Life cycle assessment (LCA) has established itself as the dominant method for identifying the environmental impact of products or services. However, conducting an LCA is labor and time intensive (especially regarding data collection). This paper, therefore, aims to identify methods and tools that enhance the practicability of LCA, especially with regard to product complexity and variance. To this end, an initial literature review on the LCA of complex products was conducted to identify commonly cited barriers and potential solutions. The obtained information was used to derive search strategies for a subsequent comprehensive and systematic literature review of approaches that address the identified barriers and facilitate the LCA process. We identified five approaches to address the barriers of time and effort, complexity, and data intensity. These are the parametric approach, modular approach, automation, aggregation/grouping, and screening. For each, the concept as well as the associated advantages and disadvantages are described. Especially, the automated calculation of results as well as the automated generation of life cycle inventory (LCI) data exhibit great potential for simplification. We provide an overview of common LCA software and databases and evaluate the respective interfaces. As it was not considered in detail, further research should address options for automated data collection in production by utilizing sensors and intelligent interconnection of production infrastructure as well as the interpretation of the acquired data using artificial intelligence.