08 Fakultät Mathematik und Physik

Permanent URI for this collectionhttps://elib.uni-stuttgart.de/handle/11682/9

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    Quantum Fourier transform for nanoscale quantum sensing
    (2021) Vorobyov, Vadim; Zaiser, Sebastian; Abt, Nikolas; Meinel, Jonas; Dasari, Durga; Neumann, Philipp; Wrachtrup, Jörg
    The quantum Fourier transformation (QFT) is a key building block for a whole wealth of quantum algorithms. Despite its proven efficiency, only a few proof-of-principle demonstrations have been reported. Here we utilize QFT to enhance the performance of a quantum sensor. We implement the QFT algorithm in a hybrid quantum register consisting of a nitrogen-vacancy (NV) center electron spin and three nuclear spins. The QFT runs on the nuclear spins and serves to process the sensor - i.e., the NV electron spin signal. Specifically, we show the application of QFT for correlation spectroscopy, where the long correlation time benefits the use of the QFT in gaining maximum precision and dynamic range at the same time. We further point out the ability for demultiplexing the nuclear magnetic resonance (NMR) signals using QFT and demonstrate precision scaling with the number of used qubits. Our results mark the application of a complex quantum algorithm in sensing which is of particular interest for high dynamic range quantum sensing and nanoscale NMR spectroscopy experiments.
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    Magnetic domains and domain wall pinning in atomically thin CrBr3 revealed by nanoscale imaging
    (2021) Sun, Qi-Chao; Song, Tiancheng; Anderson, Eric; Brunner, Andreas; Förster, Johannes; Shalomayeva, Tetyana; Taniguchi, Takashi; Watanabe, Kenji; Gräfe, Joachim; Stöhr, Rainer; Xu, Xiaodong; Wrachtrup, Jörg
    The emergence of atomically thin van der Waals magnets provides a new platform for the studies of two-dimensional magnetism and its applications. However, the widely used measurement methods in recent studies cannot provide quantitative information of the magnetization nor achieve nanoscale spatial resolution. These capabilities are essential to explore the rich properties of magnetic domains and spin textures. Here, we employ cryogenic scanning magnetometry using a single-electron spin of a nitrogen-vacancy center in a diamond probe to unambiguously prove the existence of magnetic domains and study their dynamics in atomically thin CrBr3. By controlling the magnetic domain evolution as a function of magnetic field, we find that the pinning effect is a dominant coercivity mechanism and determine the magnetization of a CrBr3 bilayer to be about 26 Bohr magnetons per square nanometer. The high spatial resolution of this technique enables imaging of magnetic domains and allows to locate the sites of defects that pin the domain walls and nucleate the reverse domains. Our work highlights scanning nitrogen-vacancy center magnetometry as a quantitative probe to explore nanoscale features in two-dimensional magnets.
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    Dopant-assisted stabilization of negatively charged single nitrogen-vacancy centers in phosphorus-doped diamond at low temperatures
    (2023) Geng, Jianpei; Shalomayeva, Tetyana; Gryzlova, Mariia; Mukherjee, Amlan; Santonocito, Santo; Dzhavadzade, Dzhavid; Dasari, Durga Bhaktavatsala Rao; Kato, Hiromitsu; Stöhr, Rainer; Denisenko, Andrej; Mizuochi, Norikazu; Wrachtrup, Jörg
    Charge state instabilities have been a bottleneck for the implementation of solid-state spin systems and pose a major challenge to the development of spin-based quantum technologies. Here we investigate the stabilization of negatively charged nitrogen-vacancy (NV - ) centers in phosphorus-doped diamond at liquid helium temperatures. Photoionization of phosphorous donors in conjunction with charge diffusion at the nanoscale enhances NV 0 to NV - conversion and stabilizes the NV - charge state without the need for an additional repump laser. The phosphorus-assisted stabilization is explored and confirmed both with experiments and our theoretical model. Stable photoluminescence-excitation spectra are obtained for NV - centers created during the growth. The fluorescence is continuously recorded under resonant excitation to real-time monitor the charge state and the ionization and recombination rates are extracted from time traces. We find a linear laser power dependence of the recombination rate as opposed to the conventional quadratic dependence, which is attributed to the photo-ionization of phosphorus atoms.
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    Addressing single nuclear spins quantum memories by a central electron spin
    (2022) Vorobyov, Vadim; Javadzade, Javid; Joliffe, Matthew; Kaiser, Florian; Wrachtrup, Jörg
    Nuclei surrounding single electron spins are valuable resources for quantum technology. For application in this area, one is often interested in weakly coupled nuclei with coupling strength on the order of a few 10-100 kHz. In this paper, we compare methods to address single nuclear spins with this type of hyperfine coupling to a single electron spin. To achieve the required spectral resolution, we specifically focus on two methods, namely dynamical decoupling and correlation spectroscopy. We demonstrate spectroscopy of two single nuclear spins and present a method to derive components of their hyperfine coupling tensor from those measurements.